 "Natural Act" was recorded at Sunset Sound and was produced by David Anderle, who had produced their first duet album and several solo albums since.Musically, the album leaned more to pop than rock and featured relaxed southern boogie, nostalgic pop ballads and country-tinged numbers alongside more unusual choices such as a reworking of "I Fought the Law," a hit for The Bobby Fuller Four in 1966, which found them sounding like the Everly Brothers.With the couple's marriage disintegrating, several cuts carry a wistful poignancy, such as "Love Don’t Live Here Anymore" and the two older Kristofferson compositions, "Please Don’t Tell Me How the Story Ends", which had been a hit for Ray Price, and the regretful "Loving You Was Easier (Than Anything I'll Ever Do Again)", which Willie Nelson covered the following year on his "Sings Kristofferson" LP.