 Gradually bending eastward through the town of Greenville, NY 81 intersects with the northern terminus of CR 41 (Greenville Center Road).After CR 41, NY 81 bends to the southeast once again, winding past at an intersection with CR 35 (West Road), which terminates there.Making a dart eastward, NY 81 turns to the southeast past the hamlet of Surprise, where the route becomes a rural two-lane roadway once again.